菜单
  

    13,14
    copper,
    14-16
    nickel,
    8,17
    titanium,
    16,18,19
    zirco-
    nium,
    18,20
    tantalum,
    21
    silicon,
    22,23
    mica,
    24
    silver,
    14,16
    iron,
    2,16,25
    manganese, and chromium26
    have been used as substrates to form
    SAMs. The choice of headgroup is critical for the stability of
    SAMs. Long chain aliphatic molecules with headgroups such as
    silanes,
    27,28
    thiols,
    29,30
    carboxylic acid,
    13,31-35
    phosphonic acid,
    36-39
    sulfonic acid,
    39,40
    and hydroxamic acid16,41
    have been utilized on
    (17) Quinones, R.; Raman, A.; Gawalt, E. S. Thin Solid Films 2008, 516(23),
    8774–8781.
    (18) Pawsey, S.; Yach, K.; Reven, L. Langmuir 2002, 18(13), 5205–5212.
    (19) Gawalt, E. S.; Lu, G.; Bernasek, S. L.; Schwartz, J. Langmuir 1999, 15(26),
    8929–8933.
    (20) Gao, W.; Dickinson, L.; Grozinger, C.; Morin, F. G.; Reven, L. Langmuir
    1996, 12(26), 6429–6435.
    (21) Palma, R.; Laureyn, W.; Frederix, F.; Bonroy, K.; Pireaux, J. J.; Borghs,
    G.; Maes, G. Langmuir 2007, 23(2), 443–451.
    (22) Miller, J. B.; Schwartz, J.; Bernasek, S. L. J. Am. Chem. Soc. 1993, 115(18),
    8239–8247.
    (23) Midwood, K. S.; Carolus, M. D.; Danahy, M. P.; Schwarzbauer, J. E.;
    Schwartz, J. Langmuir 2004, 20(13), 5501–5505.
    (24) Diez-Perez, I.; Luna,M.; Teheran, F.; Ogletree, D. F.; Sanz, F.; Salmeron,
    M. Langmuir 2004, 20(4), 1284–1290.
    (25) Volmer-Uebing, M.; Stratmann, M. Appl. Surf. Sci. 1992, 55(1), 19–35.
    (26) Hild, R.; David, C.; Muller, H. U.; Volkel, B.; Kayser, D. R.; Grunze, M.
    Langmuir 1998, 14(2), 342–346.
    (27) Sinapi, F.; Naji, A.; Delhalle, J.;Mekhalif, Z. Surf. Interface Anal. 2004, 36
    (11), 1484–1490.
    (28) Duwez, A. S.; Jonas, U.; Klein, H. ChemPhysChem 2003, 4(10), 1107–1111.
    (29) Mekhalif, Z. R., J.; Pireaux, J.-J.; Delhalle, J. Langmuir 1997, 13(8), 2285–
    2290.
    (30) Sung, M. M.; Sung, K.; Kim, C. G.; Lee, S. S.; Kim, Y. J. Phys. Chem. B
    2000, 104(10), 2273–2277.
    (31) Pawsey, S.; Yach,K.;Halla, J.; Reven, L. Langmuir 2000, 16(7), 3294–3303.
    (32) Raman, A.; Gawalt, E. S. Langmuir 2007, 23(5), 2284–2288.
    (33) van den Brand, J.; Blajiev,O.; Beentjes, P. C. J.; Terryn,H.; deWit, J.H.W.
    Langmuir 2004, 20(15), 6308–6317.
    (34) Lim,M. S.; Feng, K.; Chen, X. Q.;Wu, N. Q.; Raman, A.; Nightingale, J.;
    Gawalt, E. S.;Korakakis,D.;Hornak, L.A.; Timperman, A. T. Langmuir 2007, 23
    (5), 2444–2452.
    (35) Sondag, A. H. M.; Raas, M. C. J. Chem. Phys. 1989, 91, 4926–4931.
    (36) Quinones, R.; Raman, A.; Gawalt, E. S. Surf. Interface Anal. 2007, 39(7),
    593–600.
    (37) Raman, A.;Dubey,M.; Gouzman, I.; Gawalt, E. S. Langmuir 2006, 22(15),
    6469–6472.
    (38) Gawalt, E. S.; Avaltroni, M. J.; Koch, N.; Schwartz, J. Langmuir 2001, 17
    (19), 5736–5738.
    (39) Yee, C.; Kataby, G.; Ulman, A.; Prozorov, T.; White, H.; King, A.;
    Rafailovich, M.; Sokolov, J.; Gedanken, A. Langmuir 1999, 15(21), 7111–7115.
    (40) Fiurasek, P.; Reven, L. Langmuir 2007, 23(5), 2857–2866.
    (41) Telegdi, J.; Rigo, T.; Kalman, E. J. Electroanal. Chem. 2005, 582(1-2),
    191–201.these metal and metal oxide substrates. Despite a significant
    number of reports of SAMs on metal oxides, it is difficult to
    predict which headgroup or acid will result in a complete mono-
    layer on a specific metal substrate. This has been proven to be
    even more difficult on alloy oxides, where little work has been
    done.
    27,36,37,42-44
    Stainless steel 316L is a low-carbon austenitic steel which is
    used as surgical implant material. Like all stainless steels, it
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